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By Bernhard Kramer

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The diffusion of linear polymers into networks is much more complicated and no simple theory has been presented to explain any of the observed behavior. When the diffusing species is of high molecular weight, and interdiffusion cannot complete, only partial diffusion occurs. In this case there is the B. ): Adv. in Solid State Phys. 45, 29–44 (2005) c Springer-Verlag Berlin Heidelberg 2005 30 Mark Geoghegan possibility to study interdigitation between linear polymers and networks as a means of providing adhesion.

L. Aarts et al. 01 1E-3 0 2 4 6 x (mm) 8 10 12 Fig. 6. Static height-height correlation function gh (x) as obtained from quantitative analysis of LSCM pictures as a function of the (lateral) distance x for state points I, V, VI and VIII (see Fig. 3) approaching the critical point from bottom to top. 11 Fig. 7. (a) Interfacial tension γ as a function of the overall colloid packing fraction φc obtained from gh (x) (crosses: slow frame rate, pluses: fast frame rate). (b) The capillary length L as a function of φc obtained from gh (x).

Indeed, we also were able to proton irradiate these networks to cause uniform crosslinking. The swelling of both networks (chemically synthesized and irradiated) was the same; in fact the irradiation route is only suitable for lightly crosslinked networks and the chemical route more suitable for networks with a large crosslinking density, but there is an overlap region where swelling could be compared. The chemistry is fully described in the original paper [17]. To measure the swelling we floated a linear polystyrene layer onto water and picked it up on a polystyrene network (previously spin cast onto silicon) from a glass microslide.

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